Search results for "F center"

showing 4 items of 4 documents

First principles hybrid Hartree-Fock-DFT calculations of bulk and (001) surface F centers in oxide perovskites and alkaline-earth fluorides

2020

Valuable discussions with E. A. Kotomin are gratefully acknowledged. Research contribution of R. E. and A. I. P. has been performed within the framework of the EUROfusion Enabling Research project: ENR-MFE19.ISSP-UL-02 “Advanced experimental and theoretical analysis of defect evolution and structural disordering in optical and dielectric materials for fusion applications.” The views and opinions expressed herein do not necessarily reflect those of the European Commission.

010302 applied physicsAlkaline earth metalMaterials sciencePhysics and Astronomy (miscellaneous)F centerperovskitesGeneral Physics and AstronomyIonic bondingElectronic structure7. Clean energy01 natural sciencesCrystallographic defectCrystallographyAb initio quantum chemistry methodsVacancy defect0103 physical sciences:NATURAL SCIENCES:Physics [Research Subject Categories]Ab initio calculations010306 general physicsShallow donorPerovskite (structure)
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First principles calculations of SrZrO3 bulk and ZrO2-terminated (001) surface F centers

2016

Abstract Using a supercell model and B3PW hybrid exchange-correlation functional in the framework of the density functional theory (DFT), as it is implemented in the CRYSTAL computer code, we performed ab initio calculations for the F -center located in the SrZrO 3 bulk and on the ZrO 2 -terminated (001) surface. According to the results of performed relaxation of atoms around the defect, two nearest Zr and four Sr atoms are repulsed, but all oxygen atoms are attracted towards both, the bulk and (001) surface F -center. The displacement magnitudes of atoms surrounding the bulk F -center are smaller than around the (001) surface F -center. The B3PW calculated SrZrO 3 bulk optical band gap (5…

Band gapChemistryMaterials Science (miscellaneous)Ab initioBulk F center02 engineering and technology021001 nanoscience & nanotechnologyCondensed Matter Physics01 natural sciencesSrZrO3Electronic Optical and Magnetic Materials(001) surface F-CenterCrystalChemical bondAb initio quantum chemistry methodsVacancy defect0103 physical sciencesMaterials ChemistryDensity functional theoryAb initio calculationsAtomic physics010306 general physics0210 nano-technologyPerovskite (structure)Computational Condensed Matter
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Kinetics of dimer F2 type center annealing in MgF2 crystals

2018

Authors are greatly indebted to V. Lisitsyn, A. Ch. Lushchik and R.Vila for stimulating discussions. This work has been carried out within the framework of the EUROfusion Consortium and has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement number 633053. The views and opinions expressed herein do not necessarily reflect those of the European Commission. The calculations were performed using facilities of the Stuttgart Supercomputer Center (project DEFTD 12939).

DiffusionAnnealing kinetics:NATURAL SCIENCES:Physics [Research Subject Categories]MgF2F2 centersRadiation defectsF centers
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Kinetics of the electronic center annealing in Al2O3 crystals

2018

Authors are greatly indebted to A. Ch. Lushchik, V. Kortov, M. Izerrouken and R.Vila for stimulating discussions. This work has been carried out within the framework of the Eurofusion Consortium and has received funding from the Euroatom research and training programme 2014–2018 under grant agreement No 633053 . The views and opinions expressed herein do not necessarily reflect those of the European Commission. The calculations were performed using facilities of the Stuttgart Supercomputer Center (project DEFTD 12939 ).

Nuclear and High Energy PhysicsMaterials scienceAnnealing (metallurgy)DimerKinetics02 engineering and technology01 natural sciencesMolecular physicsF centersRadiation defectsIonDiffusionchemistry.chemical_compound0103 physical sciencesAl2O3:NATURAL SCIENCES:Physics [Research Subject Categories]General Materials Science010306 general physicsNeutron irradiationAnnealing kineticsF2 centers021001 nanoscience & nanotechnologyRecombinationNuclear Energy and Engineeringchemistry0210 nano-technologyRecombination
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